Piezoresistive properties for soft structures using hybrid CCB/CNT-based natural rubber latex composites

Abstract

This study explores the development of flexible sensors for soft structures. Conductive carbon black (CCB) and carbon nanotubes (CNT) were incorporated into a natural rubber (NR) matrix using glutaraldehyde (GA) as a curing system. The sensor properties of latex-NR composites with 20 phr of CCB, including variations of CNT content (0.5 to 3 phr), were examined. Increasing CNT content beyond 0.5 phr decreased tensile strength and elongation at break, but improved sensitivity and gauge factor (GF). Additionally, applying a voltage over 5 V caused a joule heating of the latex-NR composite strip elements. When integrated onto a soft tendon-based TPU bending actuator, higher CNT content reduced electrical signal drift during cyclic bending, enhancing long-term monitoring. This research highlights the potential of CCB/CNT-based latex-NR composites for soft structure applications, including soft robotics and health monitoring.