The regime of aerosol asymmetry parameter over Europe, Mediterranean and Middle East based on MODIS satellite data: evaluation against surface AERONET measurements

摘要

Abstract. Atmospheric particulates are a significant forcing agent for the radiative energy budget of the Earth-atmosphere system. The particulates' interaction with radiation, which defines their climate effect, is strongly dependent on their optical properties. In the present work, we study one of the most important optical properties of aerosols, the asymmetry parameter (gaer), in the region comprised of North Africa, the Arabian peninsula, Europe, and the Mediterranean basin. These areas are of great interest, because of the variety of aerosol types they host, both anthropogenic and natural. Using satellite data from the collection 051 of MODIS (MODerate resolution Imaging Spectroradiometer, Terra and Aqua), we investigate the spatio-temporal characteristics of the asymmetry parameter. We generally find significant spatial variability, with larger values over regions dominated by larger size particles, e.g. outside the Atlantic coasts of north-western Africa, where desert-dust outflow is taking place. The gaer values tend to decrease with increasing wavelength, especially over areas dominated by small particulates. The intra-annual variability is found to be small in desert-dust areas, with maximum values during summer, while in all other areas larger values are reported during the cold season and smaller during the warm. Significant intra-annual and inter-annual variability is observed around the Black Sea. However, the inter-annual trends of gaer are found to be generally small. Although satellite data have the advantage of broad geographical coverage, they have to be validated against reliable surface measurements. Therefore, we compare satellite-based values with gaer values measured at 69 stations of the global surface network AERONET (Aerosol Robotic Network), located within our region of interest. This way, we provide some insight on the quality and reliability of MODIS data. We report generally better agreement at the wavelength of 870 nm (correlation coefficient R up to 0.47) while of all wavelengths the results of the comparison were better for spring and summer.