Supplementary material

摘要

<strong class="journal-contentHeaderColor">Abstract.</strong> We derived two observation-based global monthly mean dust aerosol optical depth (DAOD) climatological datasets from 2007 to 2019 with a 2<span class="inline-formula">^∘</span> (latitude) <span class="inline-formula">×</span> 5<span class="inline-formula">^∘</span> (longitude) spatial resolution, one based on Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and the other on Moderate Resolution Imaging Spectroradiometer (MODIS) observations. In addition, the CALIOP climatological dataset also includes dust vertical extinction profiles. Dust is distinguished from non-dust aerosols based on particle shape information (e.g., lidar depolarization ratio) for CALIOP and on dust size and absorption information (e.g., fine-mode fraction, à ngström exponent, and single-scattering albedo) for MODIS, respectively. The two datasets compare reasonably well with the results reported in previous studies and the collocated Aerosol Robotic Network (AERONET) coarse-mode AOD. Based on these two datasets, we carried out a comprehensive comparative study of the spatial and temporal climatology of dust. On a multi-year average basis, the global (60<span class="inline-formula">^∘</span> S–60<span class="inline-formula">^∘</span> N) annual mean DAOD is 0.032 and 0.067 according to CALIOP and MODIS retrievals, respectively. In most dust-active regions, CALIOP DAOD generally correlates well (correlation coefficient <span class="inline-formula"><i>R</i>&gt;0.6</span>) with the MODIS DAOD, although the CALIOP value is significantly smaller. The CALIOP DAOD is 18 %, 34 %, 54 %, and 31 % smaller than MODIS DAOD over the Sahara, the tropical Atlantic Ocean, the Caribbean Sea, and the Arabian Sea, respectively. Applying a regional specific lidar ratio (LR) of 58 sr instead of the 44 sr used in the CALIOP operational retrieval reduces the difference from 18 % to 8 % over the Sahara and from 34 % to 12 % over the tropical Atlantic Ocean. However, over eastern Asia and the northwestern Pacific Ocean (NWP), the two datasets show weak correlation. Despite these discrepancies, CALIOP and MODIS show similar seasonal and interannual variations in regional DAOD. For dust aerosol over the NWP, both CALIOP and MODIS show a declining trend of DAOD at a rate of about 2 % yr<span class="inline-formula">^−1</span>. This decreasing trend is consistent with the observed declining trend of DAOD in the southern Gobi Desert at a rate of 3 % yr<span class="inline-formula">^−1</span> and 5 % yr<span class="inline-formula">^−1</span> according to CALIOP and MODIS, respectively. The decreasing trend of DAOD in the southern Gobi Desert is in turn found to be significantly correlated with increasing vegetation and decreasing surface wind speed in the area.